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Sato, Ikken; Yoshikawa, Shinji; Yamashita, Takuya; Shimomura, Kenta; Cibula, M.*; Mizokami, Shinya*
Nuclear Engineering and Design, 422, p.113088_1 - 113088_24, 2024/06
Ouchi, Kazuki
Hosha Kagaku, (49), p.3 - 7, 2024/03
I introduce the elucidation of the deposition following the oxidation state of uranium and the electrochemical behavior of uranium(IV) chloride in an ionic liquid-organic mixture, as a basic study of in-solution reactions. In addition, I introduce the development of separation methods for actinides using a microchemical chip and polyacrylamide gel electrophoresis, as an applied study for quantitative analytical methods for small amounts of samples.
He spin filter and small-angle X-ray scatteringRyoki, Akiyuki*; Watanabe, Fumi*; Okudaira, Takuya*; Takahashi, Shingo*; Oku, Takayuki; Hiroi, Kosuke; Motokawa, Ryuhei; Nakamura, Yo*
Journal of Chemical Physics, 160(11), p.114907_1 - 114907_9, 2024/03
Times Cited Count：0Kamiya, Tomohiro; Yoshida, Hiroyuki
Proceedings of the Symposium on Shock Waves in Japan (Internet), 7 Pages, 2024/03
We developed a ghost fluid method satisfying conservation laws to simulate steam explosions that can occur at the accident of a nuclear power plant. In the developed method, a first-order approximation is applied to interface effect regions, and a high-order approximation is applied to bulk regions. In other words, the algorithm of the developed method is not consistent. Therefore, we modify the way of getting ghost fluids and propose a comprehensive algorithm that applies a high-order approximation to interface effect regions. In the presentation, we will report the outlines and results of the numerical tests of it.
Yamano, Hidemasa; Futagami, Satoshi; Ando, Masanori; Kurisaka, Kenichi
Transactions of the 27th International Conference on Structural Mechanics in Reactor Technology (SMiRT 27) (Internet), 11 Pages, 2024/03
In this study, the dynamic structural analysis of the reactor vessel for excessive earthquake using the FINAS/STAR code has shown the elephant foot buckling deformation and calculated the cumulative fatigue failure fraction. Using the calculation results, this paper describes the fragility curve using the safety factor method, indicating the significantly improved curve compared the previous one.
Yamaguchi, Yoshihito; Mano, Akihiro; Li, Y.
Transactions of the 27th International Conference on Structural Mechanics in Reactor Technology (SMiRT 27) (Internet), 10 Pages, 2024/03
The steam generator (SG) is an important component of a pressurized water reactor. In addition, local wall-thinning has been reported in SG tubes. The burst differential pressure, considering both the internal and external pressures from the primary and secondary coolant systems, should be predicted for the failure probability evaluation or structural integrity assessment of SG tubes. In this study, based on the results of burst tests performed in Japan and the United States, we improved the existing burst pressure estimation method for SG tubes with wall-thinning. In addition, as an example of the utilization of the improved burst pressure estimation method, the conditional failure probabilities for SG tubes with local wall-thinning, which is necessary for probabilistic risk assessment and risk-informed decision making, are calculated considering the dimensions of the wall-thinning.
Kasahara, Naoto*; Yamano, Hidemasa; Nakamura, Izumi*; Demachi, Kazuyuki*; Sato, Takuya*; Ichimiya, Masakazu*
Transactions of the 27th International Conference on Structural Mechanics in Reactor Technology (SMiRT 27) (Internet), 8 Pages, 2024/03
In this study, we propose failure mitigation methods by application of passive safety structures. The idea of the passive safety structures was applied to next generation fast reactors under high temperature conditions and excessive earthquake conditions.
FCC hierarchical martensite transformation under dynamic impact in FeMnAlNiTi alloyLi, C.*; Fang, W.*; Yu, H. Y.*; Peng, T.*; Yao, Z. T.*; Liu, W. G.*; Zhang, X.*; Xu, P. G.; Yin, F.*
Materials Science & Engineering A, 892, p.146096_1 - 146096_11, 2024/02
Times Cited Count：0 Percentile：0.02(Nanoscience & Nanotechnology)Takai, Shizuka; Shimada, Taro; Takeda, Seiji; Koike, Katsuaki*
Mathematical Geosciences, 56(2), p.333 - 360, 2024/02
Times Cited Count：0 Percentile：0.01(Geosciences, Multidisciplinary)To enable proper remediation of accidental groundwater contamination, the contaminant plume evolution needs to be accurately estimated. In the estimation, uncertainties in both the contaminant source and hydrogeological structure should be considered, especially the temporal release history and hydraulic transmissivity. Although the release history can be estimated using geostatistical approaches, previous studies use the deterministic hydraulic property field. Geostatistical approaches can also effectively estimate an unknown heterogeneous transmissivity field via the joint data use, such as a combination of hydraulic head and tracer data. However, tracer tests implemented over a contaminated area necessarily disturb the in situ condition of the contamination. Conversely, measurements of the transient concentration data over an area are possible and can preserve the conditions. Accordingly, this study develops a geostatistical method for the joint clarification of contaminant plume and transmissivity distributions using both head and contaminant concentration data. The applicability and effectiveness of the proposed method are demonstrated through two numerical experiments assuming a two-dimensional heterogenous confined aquifer. The use of contaminant concentration data is key to accurate estimation of the transmissivity. The accuracy of the proposed method using both head and concentration data was verified achieving a high linear correlation coefficient of 0.97 between the true and estimated concentrations for both experiments, which was 0.67 or more than the results using only the head data. Furthermore, the uncertainty of the contaminant plume evolution was successfully evaluated by considering the uncertainties of both the initial plume and the transmissivity distributions, based on their conditional realizations.
Maruyama, Shuhei; Endo, Tomohiro*; Yamamoto, Akio*
Journal of Nuclear Science and Technology, 61(1), p.31 - 43, 2024/01
Times Cited Count：0 Percentile：0.01(Nuclear Science & Technology)This study investigated the feasibility of reducing the uncertainty associated with fast-reactor-core design by sharing an experimental database between different fields (e.g., reactor physics and radiation shielding) using data assimilation techniques. As the first step in this study, we focused on the ORNL sodium shielding experiment and investigated the possibility of using the experimental data to reduce the uncertainty in sodium void reactivity (SVR), which is the most important safety parameter for sodium-cooled fast reactors. A sensitivity analysis based on the Generalized Perturbation Theory was performed for the sodium shielding experiment. Using the sensitivity coefficients evaluated here and those of the sodium void reactivity previously evaluated by the JAEA, we showed that sodium shielding experimental data can contribute to the uncertainty reduction of SVR by adopting the cross-section adjustment method. Based on this study, the uncertainty reduction effect is expected to be significant, especially for SVR dominated by neutron-leakage phenomena. Although new reactor physics experimental data on SVR may be difficult to obtain, the results of this study suggest that data from sodium shielding experiments can partially substitute for this role. This study demonstrated the value of the mutual use of integral experimental data in fast reactor designs.
Zhou, L.*; Zhang, H.*; Qin, T. Y.*; Hu, F. F.*; Xu, P. G.; Ao, N.*; Su, Y. H.; He, L. H.*; Li, X. H.*; Zhang, J. R.*; et al.
Metallurgical and Materials Transactions A, 11 Pages, 2024/00
Times Cited Count：0 Percentile：0.02(Materials Science, Multidisciplinary)Soma, Shu; Ishigaki, Masahiro*; Abe, Satoshi; Shibamoto, Yasuteru
Nuclear Engineering and Technology, 10 Pages, 2024/00
Sekine, Yurina
Cellulose Communications, 30(4), p.203 - 208, 2023/12
In this paper, we introduce the fabrication and properties of carboxymethyl cellulose nanofiber (CMCF) hydrogels with high compression recoverability, macroporosity, and nontoxic properties by utilizing the phase separation phenomenon of ice crystals and solutes that occurs during freezing of aqueous solutions. The features of the developed freeze cross-linked CMCF hydrogel include that it can be made from harmless raw materials with simple procedure, high water content, and biodegradability. By taking advantage of these properties, this hydrogel synthesis technique can contribute to expanding the use of cellulose derivatives as environmental purifiers, functional materials, etc.
neutron diffractionKobayashi, Hiroki*; Komatsu, Kazuki*; Ito, Hayate*; Machida, Shinichi*; Hattori, Takanori; Kagi, Hiroyuki*
Journal of Physical Chemistry Letters (Internet), 14(47), p.10664 - 10669, 2023/11
Times Cited Count：1 Percentile：0.01(Chemistry, Physical)Ice IV is a metastable high-pressure phase of ice in which the water molecules exhibit orientational disorder. Although orientational ordering is commonly observed for other ice phases, it has not been reported for ice IV. We conducted powder neutron diffraction experiments for DCl-doped D
O ice IV to investigate hydrogen ordering in ice IV. We found abrupt changes in the temperature derivative of unit cell volume, dV/dT, at about 120 K, and revealed their slightly ordered structure at low temperatures based on the Rietveld method. The occupancy of the D1 site deviates from 0.5; it increased when samples were cooled at higher pressures and reached 0.282(5) at 2.38 GPa, 58 K. Our results evidence the presence of a low-symmetry hydrogen-ordered state corresponding to ice IV. It seems, however, difficult to experimentally access the completely ordered phase corresponding to ice IV by slow cooling at high pressure.
Higa, Ryota*; Fujihara, Hiro*; Toda, Hiroyuki*; Kobayashi, Masakazu*; Ebihara, Kenichi; Takeuchi, Akihisa*
Keikinzoku, 73(11), p.530 - 536, 2023/11
In Al-Zn-Mg alloys, suppression of hydrogen embrittlement is necessary to improve their strength. In this study, the distribution of stress, strain, and hydrogen concentration in the actual fracture region was investigated using the crystal plasticity finite element method and hydrogen diffusion analysis based on a model derived from three-dimensional polycrystalline microstructural data obtained by X-ray CT. In addition, the distributions of stress, strain, and hydrogen concentration were compared with the actual crack initiation behavior by combining in-situ observation of tensile tests using X-ray CT and simulation. The results show that stress loading perpendicular to the grain boundary due to crystal plasticity dominates grain boundary crack initiation. It was also found that internal hydrogen accumulation due to crystal plasticity has little effect on crack initiation.
Fukuda, Kodai; Yamane, Yuichi
Proceedings of 12th International Conference on Nuclear Criticality Safety (ICNC2023) (Internet), 9 Pages, 2023/10
This study presents the results of multiphysics analysis, which investigates the change of reactivity caused by the motion of fluids, of Windscale Works criticality accident. The purpose of this study is to confirm previously reported trends of emulsion formation and increase in reactivity by the multi-physics analysis which takes the motion of fluids into account. Continuous energy Monte Carlo code MVP3 was used to calculate reactivity based on the material distribution obtained by CFD calculation using OpenFOAM. An interface program in python was developed to transfer data from OpenFOAM to MVP3. The change of reactivity caused by the motion of solutions was calculated without considering the generation of heat by fissions in a system that simulated the transfer vessel at Windscale Works. As a result, trends of emulsion formation and increase in reactivity were confirmed. The influence of the resolution of the calculation system on the results was also discussed.
Kawaguchi, Maho*; Shiba, Shigeki*; Iwahashi, Daiki*; Okawa, Tsuyoshi*; Gunji, Satoshi; Izawa, Kazuhiko; Suyama, Kenya
Proceedings of 12th International Conference on Nuclear Criticality Safety (ICNC2023) (Internet), 8 Pages, 2023/10
The Nuclear Regulation Authority (NRA) has been working on an experimental approach for evaluating the criticality of fuel debris produced by the Fukushima Daiichi Nuclear Power Plant (FDNP) accident since 2014, collaborating with the Japan Atomic Energy Agency (JAEA). As part of the approach, JAEA has modified the STAtic experiment Critical facilitY (STACY) for critical experiments to evaluate characteriscs of pseudo-fuel debris. As the preliminary analyses, we verified critical characteristics with major nuclear data libraries for the proposed core configuration patterns. The three-dimensional continuous-energy Monte Carlo neutron and photon transport code, SERPENT-V2.2.0 was used with the latest JENDL, JENDL-5. As a result, larger multiplication factors of JENDL-5 across the modified STACY core configuration patterns were evaluated in comparison to the other libraries. And, 
H scattering and 
U fission sensitivity coefficients of JENDL-5 were different from those of the other libraries. Comparing among analyses with those libraries, the updated S(
, 
) of JENDL-5 might affect the result of critical characteristics in the critical analyses for the modified STACY core configuration.
Chiba, Kaori*; Matsui, Takuro*; Chatake, Toshiyuki*; Ohara, Takashi; Tanaka, Ichiro*; Yutani, Katsuhide*; Niimura, Nobuo*
Protein Science, 32(10), p.e4765_1 - e4765_13, 2023/10
Times Cited Count：0 Percentile：0(Biochemistry & Molecular Biology)Doda, Norihiro; Igawa, Kenichi*; Iwasaki, Takashi*; Murakami, Satoshi*; Tanaka, Masaaki
Nuclear Engineering and Design, 410, p.112377_1 - 112377_15, 2023/08
Times Cited Count：0 Percentile：0.01(Nuclear Science & Technology)To enhance the safety of sodium-cooled fast reactors, the decay heat in the core must be removed by natural circulation even if the AC power supply to the forced circulation equipment is lost. Under natural circulation conditions, sodium flow is driven by buoyancy, and flow velocity and temperature distribution influence each other. Thus, it is difficult to evaluate the core hot spot temperature by deterministically considering the uncertainties affecting flow and heat. In this study, a statistical evaluation method is developed for the core hot spot temperature by using Monte Carlo sampling methods. The applicability of the core hotspot evaluation method was confirmed in three representative events during natural circulation decay heat removal operations in loop-type sodium-cooled fast reactors.
Ikusawa, Yoshihisa; Nagayama, Masahiro*
JAEA-Data/Code 2023-006, 24 Pages, 2023/07
JAEA-Data-Code-2023-006.pdf:1.42MB
Core fuels with stainless steel cladding and high plutonium content mixed oxide (MOX) fuel in a water-cooled environment, such as supercritical water-cooled reactors (SCWR) and reduced-moderation water reactors (RMWR), have been studied. In order to contribute to the research and development of such a core fuel concept, the fuel performance code "FEMAXI-8" was verified based on the results of post irradiation examinations of MOX fuel irradiated in the experimental fast reactor "JOYO". FEMAXI-8 is the latest version of the behavior analysis code developed by JAEA to analyze the behavior of light water reactor fuels under normal operation and transient conditions. This latest code has been improved and developed to allow the selection of stainless steel cladding property models to analyze improved fuels such as accident tolerant fuels. The purpose of this report is to confirm the prediction accuracy of FEMAXI-8 for the irradiation behavior of the new type of core fuel that is currently being developed. As a result of the verification, it was confirmed that FEMAXI-8 has sufficient analysis accuracy for the irradiation behavior of sodium-cooled fast reactor MOX fuel with stainless steel cladding, which exceeds the plutonium content and irradiation conditions of light water reactors. In the future, the analysis accuracy of FEMAXI-8 could be improved by adopting the O/M ratio dependence of MOX fuel thermal conductivity and the irradiation behavior evaluation model at high temperature.
